Time-Resolved Research (XSD-TRR)

 
04.18.2016
Thin films are ubiquitous in computer chips and other electronic devices. Researchers have recently begun tuning the properties of these films by growing them on substrates with different crystal stru...
11-ID-D
09.14.2016
Humans can learn a lot from plants. With energy from the sun, protein catalysts in plants efficiently split water to generate oxygen, storing the energy as carbohydrates. Scientists would like to perf...
11-ID-D
09.11.2017
Researchers utilizing intense x-ray beams from the U.S. Department of Energy’s Advanced Photon Source (APS) examined the flow of electricity through semiconductors and uncovered another reason these...
10-ID-B, 11-ID-D, 12-ID-B
03.20.2019
"Frustration" plus a pulse of laser light resulted in a stable "supercrystal" created by a team of researchers from two U.S. universities and three U.S. Department of Energy national laboratories, inc...
7-ID-B,C,D, 11-ID-D, 33-BM-C, 33-ID-D,E
09.01.2020
Developing hydrogen as a fuel is important for both economic and environmental reasons. This work carried out at the U.S. Department of Energy’s Advanced Photon Source advances our understanding ...
9-BM-B,C, 11-ID-D
06.28.2021
Ultrafast X-rays Track Charge Flows in a Promising Photovoltaic Material: A class of materials known as lead halide perovskites show remarkable potential for use in optoelectronic applications. Experi...
11-ID-D
01.24.2023
Laser Excitation Alters the Structure and Light Emission of Perovskite Thin Films: Hybrid organic-inorganic perovskites show exceptional promise for use in multiple optoelectronic applications. Resea...
11-ID-D
03.06.2018
Summary here...
7-ID-B,C,D
03.14.2019
A team of researchers at the U.S. Department of Energy’s Argonne National Laboratory has developed another way of accessing ultrafast time scales by using microelectromechanical system (MEMS)-based ...
7-ID-B,C,D
03.20.2019
A team of researchers at the U.S. Department of Energy’s Argonne National Laboratory has developed another way of accessing ultrafast time scales by using microelectromechanical system-based photoni...
7-ID-B,C,D
07.08.2020
Scientists from the U.S. Department of Energy’s Advanced Photon Source have demonstrated a new research technique that address a broad range of questions concerning nanostructures of ultra-thin film...
7-ID-B,C,D
01.11.2021
Scientists using the U.S. Department of Energy's Advanced Photon Source show that hydrated starch granules mixed into conventional hydrogels can create tissue-like materials that could someday be used...
2-BM-A,B, 7-ID-B,C,D
04.20.2021
Tiny Chip-Based Device Performs Ultrafast Manipulation of X-Rays: Researchers from the U.S. Department of Energy’s Advanced Photon Source and Center for Nanoscale Materials have developed and demon...
7-ID-B,C,D
10.19.2023
Scientists who work on the production of renewable energy want to understand the photochemical processes involved in the photocatalytic production of hydrogen or the conversion of carbon dioxide into ...
7-ID-B,C,D
11.14.2023
Maximizing the energy we extract from each gallon of oil is a powerful way to conserve energy and lower our society’s carbon footprint. Scientists have used the Advanced Photon Source to directly ch...
7-ID-B,C,D
 

The TRR group has operational responsibility for undulator end stations 7-ID-B, 7-ID-C, 7-ID-D, and 25-ID-E. Time-resolved pump-probe techniques using, most often, high-power lasers as the pump, are performed in stations 7-ID-C and 7-ID-D and 25-ID-E. 7-ID-B is white-beam capable and hosts experiments that probe ultrafast fluid dynamics in high-pressure, high velocity sprays.  In addition to the x-ray-beamlines, our group maintains and enhances high-power ultrafast laser systems at 7-ID and 25-ID.

BEAMLINES
7-ID-B
7-ID-B is a white-beam-capable station primarily used for ultra-fast imaging of high density and high-speed sprays. Unique imaging capabilities include the ability to image the internal motion of operating fuel injectors and to perform single-x-ray-shot imaging of dense sprays.
7-ID-C
7-ID-C has dedicated diffraction and nanoprobe diffraction set-ups that provide Å resolution (reciprocal space) ultrafast time-resolved measurements of pumped materials. Pumps include an ultrafast high-power laser beam with 1 kHz rep-rate, an available high-rep-rate (54 kHz - 6.5 MHz) high-power laser, and terahertz (THz) radiation. Typical x-ray-beam sizes are 50 μm for samples mounted on a large 6-circle Huber diffractometer while a new zone-plate set-up provides 300 nm resolution for samples mounted on a compact Huber diffractometer. A variety of sample environments are available. Work in this station is relevant to a fundamental understanding of excitations and phase diagrams of emerging complex materials.
7-ID-D
7-ID-D is primarily devoted to pump-probe studies of ultrafast transient states of photoactive molecules in solution via the time-resolved incarnations of x-ray techniques such as XANES, EXAFS, x-ray emission (XES) spectroscopy and x-ray diffuse scattering (XDS). An ultrafast high-rep-rate (54 kHz - 6.5 MHz), high-power laser is typically used as the pump. Novel x-ray emission spectrometers are being developed and deployed that, combined with the high-rep-rate laser beams, allow the excited states of small and dilute quantities of designer photoactive molecules to be probed with high fidelity. Work performed in 7-ID-D is relevant to the fundamental understanding of photochemistry with ultimate application to artificial photosynthesis. Much of the work in this station is performed in collaboration with the CSE-AMO group.
Laser Systems
Specifications below provide general guidelines. Specific capabilities and requirements should be discussed with the beamline staff.
System Station Rep-rate Pulse
Length
Wavelength Energy per
Pulse
Ti:Sapph 7-ID-C, 7-ID-D 1 kHz 100 fs 800, 400 nm 200 μJ
Ti:Sapph with OPA 7-ID-C 1 kHz 100 fs 200nm - 20 μm 10 μJ
Duetto* 7-ID-D 54 kHz - 6.5 MHz 10 ps 1 or 0.5 μm 10 μJ
Ti:Sapph 11-ID-D 10 kHz 1.6 ps 800, 400, 266 nm 700 μJ
Ti:Sapph with OPA 11-ID-D 3 kHz 100 fs 260 nm-2.5 μm 100 μJ

Comments:
*Portable system primarily operated and maintained by CSE-AMO in Station 7-ID-D. Available for use in other stations via collaboration or permission of CSE-AMO group and with appropriate safety considerations.